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Colloquium : Water’s controversial glass transitions
ISSN
1539-0756
0034-6861
Date Issued
2016
Author(s)
DOI
10.1103/RevModPhys.88.011002
Abstract
Water is the most common and, judged from its numerous anomalous properties, the weirdest of all known liquids and the complexity of its pressure-temperature map is unsurpassed. A major obstacle on the way to a full understanding of water's structure and dynamics is the hard-to-explore territory within this map, colloquially named the no man's land. Many experiments suggest that just before stepping across its low-temperature border, amorphous ices undergo glass-to-liquid transitions while other interpretations emphasize the importance of underlying disordered (nano) crystalline states. Prospects for reconciling the conflicting views regarding the nature of water's glass transitions are discussed.