Real-time monitoring of aerosol particle formation from sulfuric acid vapor at elevated concentrations and temperatures

ISSN
1463-9076
Date Issued
2022
Author(s)
Becker, Daniel
Heitland, Jonas
Carlsson, Philip T. M.
Elm, Jonas
Olenius, Tinja
Tödter, Sophia
Kharrazizadeh, Amir
DOI
10.1039/D1CP04580F
Abstract
A new experiment enables monitoring of particles formed from highly supersaturated sulfuric acid vapor. From kinetic simulations and DLPNO-CCSD(T 0 )-calculations cluster decomposition rates in the temperature range from 296 to 325 K are deduced.