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Direct Access to Auger recombination in Graphene
Date Issued
2020-11-26
Author(s)
Keunecke, Marius
Schmitt, David
Weber, Marius
Möller, Christina
Mishra, Tridev A.
Osterkorn, Alexander
Bennecke, Wiebke
Pierz, Klaus
Schumacher, Hans Werner
Pakdehi, Davood Momeni
Steil, Daniel
Manmana, Salvatore R.
Steil, Sabine
Schneider, Hans Christian
Mathias, Stefan
Abstract
Auger scattering channels are of fundamental importance to describe and understand the non-equilibrium charge carrier dynamics in graphene. While impact excitation increases the number of carriers in the conduction band and has been observed experimentally, direct access to its inverse process, Auger recombination, has so far been elusive. Here, we tackle this problem by applying our novel setup for ultrafast time-resolved photoelectron momentum microscopy. Our approach gives simultaneous access to charge carrier dynamics at all energies and in-plane momenta within the linearly dispersive Dirac cones. We thus provide direct evidence for Auger recombination on a sub-10~fs timescale by identifying transient energy- and momentum-dependent populations far above the excitation energy. We compare our results with model calculations of scattering processes in the Dirac cone to support our experimental findings.